The 2000–01 season marked Sydney United's eighteenth campaign in the NSL. The team finished in 10th place, missing out on the final series for a second consecutive season.
Following a disappointing 1999–2000, Sydney United appointed former player Alan Hunter as head coach in an effort to revitalize the squad, along with key signings including former Australian internationals Francis Awaritefe and Zlatko Arambasic. 
The season began on a promising note, with United securing victories in their first three matches. However, a challenging period followed, as the team remained winless for the next ten games, leading to Hunter's departure. Velimir Kuprešak took over as player-coach, and while results improved under his leadership, United ultimately fell short of a finals berth. 
Additionally, the campaign marked the conclusion of Velimir Kuprešak's distinguished tenure at the club, as he retired at the end of the season, having been with Sydney United since 1989.
A standout moment of the season was the guest appearance of Croatian international Aljoša Asanović, who featured in the final two matches, scoring one goal. 
Statistics.
Appearances and goals.
Players with no appearances not included in the list.